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The Workshop addresses the use of Free-Electron Lasers (FEL) for probing structural and dynamical properties of matter at the nanoscale, and the necessary developments in experimental and theoretical methods. As novel FEL research infrastructures are coming online, efforts are urgently required in order to carry out successful science programmes. This implies an overarching approach to the understanding of all experimental aspects, from pulse structure to sample delivery to detector response, and of the theoretical tools and methods for data analysis and interpretation.