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The synergy of electronic structure theory and spectroscopic methods is transforming modern chemistry, enabling cutting-edge research across all fields of molecular science. Our highly successful series of summer schools on Molecular Theory and Spectroscopy has specifically addressed the connection between spectroscopic techniques and quantum chemical methods for the study of molecular systems. This unified approach will be again central in the 2016 edition of our summer school. This year, however, we also expand the content of our program in an effort to bridge the historic divide between homogeneous and heterogeneous catalysis.